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The Heterogeneous Electron Transfer of Cytochrome C Adsorbed on Ag Electrodes Coated with Omega-carboxyl Alkanethiols. A Surface Enhanced Resonance Raman Spectroscopic Study
Citation key ISI:000169235600017
Author Murgida, D H and Hildebrandt, P
Pages 97-100
Year 2001
ISSN 0022-2860
Address PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
Journal J. Mol. Struct.
Volume 565
Number Sp. Iss. SI
Month MAY 30
Note XXVth European Congress on Molecular Spectroscopy, COIMBRA, PORTUGAL, AUG 27-SEP 01, 2000
Publisher ELSEVIER SCIENCE BV
Abstract Cytochrome c adsorbed on Ag electrodes coated with self-assembled monolayers of carboxyl-terminated alkanethiols was studied by surface enhanced resonance Raman spectroscopy. Potential-dependent measurements indicate that the bound protein can adopt different orientations depending on protein-protein interactions and anion binding. At high protein coverage or in the presence of specifically adsorbed anions the heterogeneous distribution of orientations is responsible for the apparent non-ideal electrochemical behaviour. (C) 2001 Elsevier Science B.V. All rights reserved.
Bibtex Type of Publication Proceedings Paper
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